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Generic Schemes for Single-Molecule Kinetics. 1: Self-Consistent Pathway Solutions for Renewal Processes
Single-Molecule Kinetics Self-Consistent Pathway Solutions Renewal Processes
2014/9/24
In this paper, we discuss a strategy for reducing a complex single molecule kinetic process to a set of generic structures (motifs) that are building blocks for a general kinetic scheme. In general, t...
Single molecule kinetics. II. Numerical Bayesian approach
Single molecule kinetics Numerical Bayesian approach
2014/9/24
As discussed in the companion paper@J. B. Witkoskie and J. S. Cao, J. Chem. Phys.121, 6361~2004!, preceding paper#, quantitative extraction of information from single molecule experiments by several p...
Single molecule kinetics. I. Theoretical analysis of indicators
Single molecule kinetics Theoretical analysis
2014/9/24
Single molecule experiments reveal intriguing phenomenon in chemical and biological systems.Several indicators of complex dynamics, including ‘‘intensity’’ correlations, ‘‘event’’ correlations,and cha...
Direct measurements of memory effects in single-molecule kinetics
Direct measurements memory effects single-molecule kinetics
2014/9/24
Statistics and correlations of single-molecule sequences of modulated reactions are explicitly evaluated in the stochastic rate representation. The memory function, introduced through the Gaussian app...
Two-Event Echos in Single-Molecule Kinetics: A Signature of Conformational Fluctuations
Two-Event Echoes Single-Molecule Kinetics A Signature of Conformational Fluctuations
2014/9/24
The relationship between event-averaged measurements and ensemble averaged measurements can be clarified by averaging along single-molecule trajectories. As a result, phenomenological chemical kinetic...
Event-averaged measurements of single-molecule kinetics
Event-averaged measurements single-molecule kinetics
2014/9/24
A modulated N-conformational-channel reactive system is used to model the recent single-molecule enzymatic experiw .x ment Science 282 1998 1877 . Kinetic analysis of the model system clearly demonst...